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Third-party "portable" versions found online carry significant risks:

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Because it doesn't write to the Windows Registry in the same way an installation does, it leaves the host computer "clean". One-Time Use: microsoft office ltsc pro plus 2021 portable

Office LTSC Professional Plus 2021 includes the classic desktop versions of the following applications: Outlook for email and calendar management Publisher and Access (available for Windows only) Microsoft Teams and OneNote Key Differences from Microsoft 365 Deploy Office Long Term Service Channel (LTSC) 2021 microsoft office ltsc pro plus 2021 portable